Abstract

The deuterium and oxygen 18 concentrations of water evaporating into air of nonzero humidity do not follow the simple batch distillation equation but increase asymptotically to a stationary isotopic state as the mass of water decreases to zero. This effect is due to a rapid molecular exchange between liquid and vapor, which predominates over the simple separation effect of removal of vapor. In diy air the batch distillation law is obeyed, and the isotopic enrichment continually increases; however, the separation factor is larger than the equilibrium isotopic vapor pressure ratio when the evaporation rate is comparable to natural rates. The HDO and H2O18 enrichments in our experiments show a linear correlation with a slope of about 5.5, as found in the evaporation of natural water bodies. The mechanism of the molecular exchange will be described in following papers.

Number of times cited: 186

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